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Mauna Loa Observatory (MLO)
MLO in Hawaii "is a premier atmospheric research facility that has been continuously monitoring and collecting data related to atmospheric change since the 1950's." Features live cameras, data (carbon cycle, weather, and more), a history of the observatory, and a link to material about the 50th anniversary in November 2007 of MLO and of carbon dioxide measurement (as begun by Charles David Keeling in 1958). From the National Oceanic and Atmospheric Administration (NOAA).
http://www.mlo.noaa.gov/

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